I kinda doubt it... Maybe If when you connect to someone who's zune is connected to their xbl account, It could show their gamertag with achievements. But earning achievements on zune... no... 99% ssure it won't happen...
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When the battle of the zunes/ipods began, Apple said Give them what they want; smaller players 4 more money" Microsoft bravely stepped in and said "Give them what they Really Want; a better player with updates for free"
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